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This dissertation, through a systematic §investigation of the behavior of the gas-phase §dynamics of§nanoparticles generated by laser ablation of solid §target materials in background gases§and a study of the physical processes involved in §gas-phase nanoparticle processing, explores the §combination of laser and aerosol processes as a §novel approach to make thin§film materials with a level of microscopic §organization similar to that found in nature.§The integrated laser-aerosol method is very flexible §and can be used in the§synthesis of a variety of materials. In this study §it is applied to the deposition of§nanocomposite thin films comprising tetrahedral §amorphous carbon (ta-C) with§embedded metal nanoparticles. The controlled §incorporation of metal nanoparticles§enables the modulation of the electrical §conductivity of ta-C over four orders of§magnitude without significantly or adversely §affecting its mechanical properties.
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